I'd like to know if there is something I can do to close the gap or hide the gap in the blinds. Obviously, I can measure properly and purchase new ones but really trying to avoid that.
I've also thought about curtains, but it's also something I'd like to avoid. Are there any solutions to this?
Here is another photo zoomed out. 
I've thought about moving them closer. I can do it without issue - I suppose I can try it out and see how it looks.
You can also add sheer curtains in front of them if light is coming through. I find blinds alone are never enough.